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- 4114 discussions
hi all,
Here is a gif of Nb2O5 at Nb K-edge and TiO2 at Ti K-edge. Both
collected withb same geometry and detectors and same BL (SSRL 11-2).
Fluo was collected at 90° to the beam (while transmission data was
collected on the exact same sample).
both spectra are normalized. Is there not any remaining
self-absorption in the fluo spectrum for Nb2O5, despite data
collected at 90° ?? (while TiO2 sounds fine, as Troeger predicted ?).
thank for your expertise !
--
Francois FARGES
Laboratoire des Géomatériaux
Université de Marne la Vallée
5 Bd Descartes-Champs S/Marne
77454 Marne la Vallée cedex 2
TEL: 01 49 32 90 57
from outside France: +33 1 49 32 90 57
FAX: 01 49 32 91 37
from outside France: +33 1 49 32 91 37
3
3
Hi Everyone,
There were several conversations around the XAFS 12 conference on
self-absorption corrections for EXAFS. It would be nice to add such
corrections (and others, like for deadtime corrections) to Ifeffit.
Corwin Booth (at LBL lab, Berkeley) presented a very nice procedure
for making these corrections for EXAFS at the conference, improving
the work of L. Troger, et al from the mid 1990's. Corwin just sent
me the Fortran source code for his program so that it might be
included in Ifeffit, and is letting me pass it on. I put the source
code (with a Unix Makefile and some instructions) at
http://cars.uchicago.edu/ifeffit/contrib/sabcor.tar.gz
with a README at
http://cars.uchicago.edu/ifeffit/contrib/README.SABCOR
I'd be interested in hearing others opinions on this topic, and
whether this should be included in Ifeffit. A self-absorption
correction that worked better for XANES would be useful too. If
you've thought about self-absorption corrections or have some data
affected by self-absorption corrections, please check out Corwin's
code and let us know what you think of this.
Speaking of things to check out, Francois Farges recently created
a web page discussingCauchy Wavelet transforms of EXAFS data at
http://www.univ-mlv.fr/~farges/wav/
The site includes MATLAB code and references. These transforms are
very interesting and I recommend checking out this stuff. There was
also a recent email from Harald Funke sent to many people about a
different code for Wavelet transforms. If I get permission from
Harald, I'll post these codes too.
Related to all this, I added a 'Contributions' page to the Ifeffit
Web Pages, for "contributions and/or things to consider for XAFS
analysis and Ifeffit". Currently, this has links to Corwin's
self-absorption correction code, and Francois' Wavelet web page.
If anyone has any suggestions for other things to add, let me know.
Thanks,
--Matt
4
7
Hi folks,
The other day a user of ifeffit on linux asked a question that I have
seen several times now and so thought it would be prudent to explain
the situation on the mailing list. It is fairly easy to get confused
about the sequence of how things must be installed when installing
ifeffit on a unix machine for the first time. The explanation below
only applies to unix users (including, but not limited to, linux
users) and does not apply to MS Windows users. (The situation is
different for OSX users, as well, as indicated by last week's flurry
of email.)
When installing this stuff for the first time on a unix machine, the
correct sequence is:
1. install pgplot
2. install ifeffit
3. install Atoms, Athena, Artemis, GIfeffit, and/or SixPack
The easiest way to install pgplot is to use the PGPLOT_install script
that Matt supplies with the ifeffit source code tarball. Just unpack
the ifeffit tarball, cd into the build directory, and do
~> sh PGPLOT_install
before doing the "./configure; make; make install" incantation. This
script will try very hard to fetch the pgplot tarball from the web.
Once downloaded, it will unpack it, compile it, and install it
automagically. Once this is done, go ahead and install ifeffit.
In the future, when you upgrade ifeffit, it should not be necessary to
reinstall pgplot (unless, of course, you have done something to change
things on your computer in the interim).
When pgplot is installed correctly, the "./configure" step on the
installation will end with a message that says something like this:
===
=== ifeffit 1.2.1 Configuration Results:
=== linking to PGPLOT with: -L/usr/local/pgplot -lpgplot -lpng -lz
-L/usr/X11R6/lib -lX11
===
=== ready for next step: type 'make' then 'make install'
Note that in the second line it has correctly identified the location
of the pgplot installation and its library. It has also identified
several other libraries necessary for drawing stuff to the screen
under X.
If pgplot is not found on your computer, "./configure" will end with a
message like this:
===
=== ifeffit 1.2.1 Configuration Results:
=== linking to PGPLOT with:
/home/bruce/codes/ifeffit-1.2.1/src/pgstub/libnopgplot.a
===
=== ready for next step: type 'make' then 'make install'
Note that, in this case, the ifeffit library will be linked to
something called `libnopgplot.a'. This is a stub that allows ifeffit
to continue working as a data analysis tool even in the absence of
pgplot. That is, you will still be able to import and export data, do
background removals, and so, but you will not be able to plot stuff.
This seems like a good decision that Matt made -- that is, it seems
appropriate that ifeffit should still be functional even in the
absence of pgplot.
Athena and Artemis, however, will not function in the absence of
pgplot. If pgplot was not found and you did not notice that ifeffit
was linking to libnopgplot.a, then you will not realize that there is
a problem until *after* you have installed one of the GUIs and tried
to run them. At that point, the program will fail with a variety of
cryptic error messages like so:
Can't load
'/usr/lib/perl5/site_perl/5.8.0/i386-linux-thread-multi/auto/Ifeffit/Ifeffit.so'
for module Ifeffit:
/usr/lib/perl5/site_perl/5.8.0/i386-linux-thread-multi/auto/Ifeffit/Ifeffit.so:
undefined symbol: pgqndt_ at
/usr/lib/perl5/5.8.0/i386-linux-thread-multi/DynaLoader.pm line 229.
at /usr/bin/athena line 55
Compilation failed in require at /usr/bin/athena line 55.
BEGIN failed--compilation aborted at /usr/bin/athena line 59.
The common feature of these error messages is the failure to find
symbols that begin with the letters "pg", as in the 5th line of the
error message I replicated above.
If you run into this situation, the thing to do is to go back to the
beginning. Install pgplot and make sure that it got installed
correctly. Then build ifeffit *from scratch*. It is not enough just
to install pgplot. You MUST rebuild ifeffit after installing pgplot.
Once ifeffit it rebuilt, go ahead and install one or more of the
GUIs. Again, it is insufficient just to rebuild ifeffit and not to
rebuild the GUIs.
If you are careful to follow the procedure of installing pgplot, then
ifeffit, then GUIs, you should find that everything will work as
advertised.
And finally, if you have any questions or suggestions regarding
installation, don't hesitate to ask them here on the mailing list. If
you ask questions on the mailing list, then everyone can benefit by
the answer.
HTH,
Bruce
P.S. Carlo Segre is kindly packaging ifeffit into Debian package
files. This is a *great* way for people to help out with the
ifeffit project without needing to write code. If any of you
are users of Red Hat, SuSE, Mandrake, Connectiva, or any other
linux distribution (such as the über-cool Gentoo) and wanted to
contribute packages guaranteed to work on those systems, that
would be great! Just let me or Matt know and we will help you
get started. The same would be true for anyone using any of the
commercials unixes (Solaris, SGI, etc.) which have their own
packaging systems.
--
Bruce Ravel ----------------------------------- ravel(a)phys.washington.edu
Code 6134, Building 3, Room 222
Naval Research Laboratory phone: (1) 202 767 5947
Washington DC 20375, USA fax: (1) 202 767 1697
NRL Synchrotron Radiation Consortium (NRL-SRC)
Beamlines X11a, X11b, X23b, X24c, U4b
National Synchrotron Light Source
Brookhaven National Laboratory, Upton, NY 11973
My homepage: http://feff.phys.washington.edu/~ravel
EXAFS software: http://feff.phys.washington.edu/~ravel/software/exafs/
2
1
Dear friends,
just a small update for the potential scanning stuff: It works fine for one
shell. Really straightforward thanks to the ifeffit() calls. Some corrections
and I can provide you the program ;)
But there is one little thing I am thinking about, which is fairly general, I
think:
If I just have one shell, everything is fine. The program iterates through all
possible variable combinations.
But...
if I have two shells I just manage to let him vary the shells independently. I
know there must be a way to tell the algorithm that if there are 2 shells it
needs to vary each of the eight parameters against each other and not two
times the four from each shell.
I know there are some good PERL hackers around. So do you have an idea how to
do this? Recursion shurely helps - I experimented a lot with it but it still
does not do what I need it to do. Just for your convenience: I stored the
parameters in an array of hashes, so that I can have something like
$shell[0]{E0} = $something
$shell[0]{dr} = $somethingelse...
So the loop for one shell is just looping through the hashkeys of element 0 of
this array...
Thanks for your suggestions.
Cheers,
Norbert
--
Dr. rer. nat. Norbert Weiher (norbertweiher(a)yahoo.de)
Laboratory for Technical Chemistry - ETH Hönggerberg
HCI E 117 - 8093 Zürich - Phone: +41 1 63 3 48 32
3
2
Hello,
I just wanted to echo Scott's sentiments. If someone has the time and
energy to create for the Mac an executable version of the
Artemis/Athena/IFEFFIT programs (and keep them updated), I'd also be very
grateful. Being unfamiliar with Unix, I experienced the same problems as
Scott in trying to get the programs up and running on my Mac. So, I bought
a PC laptop specifically for doing data analysis with these very nice
programs.
Dean Hesterberg
**************************************************
Hi again,
>
>OK, I've reached a conclusion. For someone not currently using the
>open source UNIX tools and the like on the Mac, the project of
>getting Artemis, Athena, and IFEFFIT up and running is immense,
>because it means getting a large amount of additional infrastructure
>in place. Consider: Fink is required. Once Fink is installed, the
>x-free87-base package is required. That package, in turn, requires
>downloading 12 separate files (one-by-one, as far as I can tell). And
>that's just one part of a part of what is required (g77, pgplot,
>perl...). My estimate is that, with my lack of experience, it would
>take me a week full-time to get all this stuff working right. That's
>not a problem, of course, for people who already do development on
>the Mac and have most of this stuff set up anyway, or at least find
>uses for it other than getting the EXAFS packages to run. But it's
>too much of a time investment for me, and I suspect that the same is
>true for a lot of others in the field.
>
>So I'm going to scrounge a pc from somewhere, transfer my data files
>>from the Mac, and download the executable there.
>
>If at some point an executable appears for the Mac, I will thank the
>authors profusely...I realize that no one is getting paid to work on
>this!
>
>--Scott Calvin
>Naval Research Lab
>Code 6344
>_______________________________________________
>Ifeffit mailing list
>Ifeffit(a)millenia.cars.aps.anl.gov
>http://millenia.cars.aps.anl.gov/mailman/listinfo/ifeffit
------------------------------------------------------
DEAN HESTERBERG
Associate Professor
Department of Soil Science
College of Agriculture and Life Sciences
North Carolina State University
Box 7619 (3235 Williams Hall)
Raleigh, NC 27695-7619
E-mail: dean_hesterberg(a)ncsu.edu
FAX: (919) 515-2167 tel: (919) 513-3035
7
14
Cheers friends,
now a short question concerning reference paths calculated by FEFF (I use
FEFF8.1):
I have a series of spectra of catalysts containing V,P and O. Data was taken
at the V K edge. I know from literature, that the first coordination shell
should contain some 5-6 O atoms. The problem (and this is really the first
time I ever had problems with this) is that ifeffit (V 1.2.1) is not capable
of fitting even the first shell. As it works fine for model systems, e.g. Au
foil, I wonder if I have problems with the calculation of the references...
As first try, I re-calculated the feffxxxx.dat files with the SCF flag turned
on (which I never used before for the EXAFS) - the problem persisted. Has one
of you experienced similar problems and knows how to come over?
Norbert
--
Dr. rer. nat. Norbert Weiher (norbertweiher(a)yahoo.de)
Laboratory for Technical Chemistry - ETH Hönggerberg
HCI E 117 - 8093 Zürich - Phone: +41 1 63 3 48 32
3
2
Hi folks,
first of all thanks to all of you who attended the XAFS XII for an interesting
conference with lots of input and new ideas.
But now to my question:
I have been guessing for a long time of doing an algorithm of doing some kind
of potential surface scanning when doing an EXAFS fit. This procedure has
been known in e.g. ab initio codes like GAUSSIAN for a long time and can be
used to check if you are really in a global minimum on the potential surface.
As EXAFS analysis is the ultimate search for a global minimum in the
parameter space, but you never know if you really end up there, I was
planning to do such kind of investigations.
However, before I start off with wild coding :) I want to have more opinions
on this topic. Here are my main points speaking for this kind of algorithm:
1) Computer power is quite fast now - and ifeffit is also really fast in
computing the fit quality if you do not guess any variable (which you don't
need in this case as you vary the parameters by your own).
2) In cases where you would expect large correlations between certain
variables (e.g. when you have overlapping shells at nearly the same
distance), one could systematically investigate the influence of small
changes in the parameter space on the fit.
That's it - now I am really keen on knowing what you think of this idea.
Cheers,
Norbert
--
Dr. rer. nat. Norbert Weiher (norbertweiher(a)yahoo.de)
Laboratory for Technical Chemistry - ETH Hönggerberg
HCI E 117 - 8093 Zürich - Phone: +41 1 63 3 48 32
3
2
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--CSmtpMsgPart123X456_000_000589E5--
1
0
Hi. This is the qmail-send program at mail.hive.nj2.inquent.com.
I'm afraid I wasn't able to deliver your message to the following addresses.
This is a permanent error; I've given up. Sorry it didn't work out.
<arnold(a)beryldshannon.com>:
user is over quota
--- Below this line is a copy of the message.
Return-Path: <ifeffit(a)millenia.cars.aps.anl.gov>
Received: (qmail 28325 invoked by uid 109); 10 Jul 2003 22:44:41 -0000
Delivered-To: beryldshannon.com-webmaster(a)beryldshannon.com
Received: (qmail 28311 invoked from network); 10 Jul 2003 22:44:40 -0000
Received: from unknown (HELO COMPUTERNAME) (24.191.167.224)
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From: <ifeffit(a)millenia.cars.aps.anl.gov>
To: <webmaster(a)beryldshannon.com>
Subject: Re: Movie
Date: Thu, 10 Jul 2003 18:44:40 --0400
Importance: Normal
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--CSmtpMsgPart123X456_000_00059887
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--CSmtpMsgPart123X456_000_00059887--
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Hello, it's me again,
it was a pleasure for me to hear that IFEFFIT can now handle restraints. I
read the documentation on handling them on the IFEFFIT homepage but one thing
is still unclear:
I see how you can say that a value should be near some number you know from
other methods. But how do I apply a range? Of course, I could always use the
midpoint of the restraint interval and use the way described - but can you do
it in other ways?
The last question concerns the weighting factor: Let's keep with Matt's
example of setting a restraint on a distance to 2.54. If I use the weighting
of 0.01 shown in the example, what would be the max. and min. values the fit
can run to? Is it +/- 1 % deviation or something else?
Cheers,
Norbert
--
Dr. rer. nat. Norbert Weiher (norbertweiher(a)yahoo.de)
Laboratory for Technical Chemistry - ETH Hönggerberg
HCI E 117 - 8093 Zürich - Phone: +41 1 63 3 48 32
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