Hi Johannes,
I guess I hadn't tested the Chantler results below about 1 keV, and certainly not at 100 eV. To be clear, Chantler claims the error bars on these value of "50 to 200%" below 200 eV. But the spline interpolation is much, much worse than that!
Spline interpolation is definitely preferred at higher energies, and where the grid of tabulated data is fine enough. But we should better explore when that is valid, and/or automatically use linear interpolation below some energy, and/or allow the user to select the interpolation order.
Anyway, thanks very much. We should make this better at all energy ranges.
--Matt